иҝ‘ж—ҘпјҢжөҷжұҹеёҲиҢғеӨ§еӯҰеҗ«ж°ҹж–°жқҗж–ҷз ”з©¶жүҖиҙІи…ҫеӣўйҳҹеңЁж–°еһӢеӨҡеӯ”жқҗж–ҷи®ҫи®ЎдёҺеӨӘйҳіиғҪеӮ¬еҢ–еҲ©з”ЁйўҶеҹҹеҸ–еҫ—йҮҚиҰҒиҝӣеұ•гҖӮзӣёе…із ”з©¶жҲҗжһңд»Ҙйўҳдёә вҖңPositional Effects of SingleвҖҗAtom Active Sites in 1D Porphyrinic COFs on Photocatalytic CO2 ReductionвҖқ зҡ„з ”з©¶и®әж–ҮеҸ‘иЎЁдәҺеӣҪйҷ…еҢ–еӯҰйўҶеҹҹжңҹеҲҠ Angewandte Chemie International EditionгҖӮ
дәҢж°§еҢ–зўіпјҲCO2пјүиө„жәҗеҢ–еҲ©з”ЁжҳҜе®һзҺ°з»ҝиүІдҪҺзўіеҸ‘еұ•зҡ„йҮҚиҰҒз ”з©¶ж–№еҗ‘гҖӮеҲ©з”ЁеӨӘйҳіиғҪе°ҶCO2иҪ¬еҢ–дёәе…·жңүеә”з”Ёд»·еҖјзҡ„еҢ–еӯҰе“Ғе’ҢзҮғж–ҷпјҢиў«и®ӨдёәжҳҜи§ЈеҶіиғҪжәҗдёҺзҺҜеўғй—®йўҳзҡ„йҮҚиҰҒйҖ”еҫ„д№ӢдёҖгҖӮз„¶иҖҢпјҢCO2еҲҶеӯҗз»“жһ„зЁіе®ҡпјҢе®һзҺ°й«ҳж•ҲгҖҒй«ҳйҖүжӢ©жҖ§зҡ„иҪ¬еҢ–д»ҚйқўдёҙиҜёеӨҡжҢ‘жҲҳгҖӮеҰӮдҪ•и®ҫи®Ўй«ҳжҖ§иғҪеӮ¬еҢ–жқҗж–ҷпјҢе№¶зІҫеҮҶи°ғжҺ§еҸҚеә”иҝҮзЁӢдёӯзҡ„е…ій”®жӯҘйӘӨпјҢжҳҜиҜҘйўҶеҹҹзҡ„йҮҚиҰҒз§‘еӯҰй—®йўҳгҖӮй’ҲеҜ№дёҠиҝ°й—®йўҳпјҢиҙІи…ҫеӣўйҳҹеҸ‘еұ•дәҶдёҖз§Қж–°еһӢз»“жһ„и®ҫи®Ўзӯ–з•ҘпјҢжһ„зӯ‘дәҶдёҖзұ»е…·жңүзІҫеҮҶи°ғжҺ§жҙ»жҖ§дёӯеҝғдҪҚзҪ®зҡ„дёҖз»ҙеҚҹе•үе…ұд»·жңүжңәжЎҶжһ¶пјҲCOFпјүжқҗж–ҷгҖӮз ”з©¶еҸ‘зҺ°пјҢеӮ¬еҢ–жқҗж–ҷдёӯжҙ»жҖ§дҪҚзӮ№жүҖеӨ„зҡ„дҪҚзҪ®дјҡжҳҫи‘—еҪұе“ҚCO2иҪ¬еҢ–иҝҮзЁӢе’ҢжңҖз»Ҳдә§зү©йҖүжӢ©жҖ§гҖӮйҖҡиҝҮи°ғжҺ§й“ңжҙ»жҖ§дёӯеҝғеңЁжқҗж–ҷйӘЁжһ¶дёӯзҡ„з©әй—ҙеҲҶеёғпјҢеӣўйҳҹе®һзҺ°дәҶеҜ№CO2иҝҳеҺҹеҸҚеә”и·Ҝеҫ„зҡ„жңүж•Ҳи°ғиҠӮгҖӮ
з ”з©¶з»“жһңиЎЁжҳҺпјҢдёҚеҗҢдҪҚзҪ®зҡ„й“ңжҙ»жҖ§дёӯеҝғиЎЁзҺ°еҮәдёҚеҗҢзҡ„еӮ¬еҢ–зү№жҖ§гҖӮе…¶дёӯпјҢдҪҚдәҺжқҗж–ҷдёӯеҝғеҢәеҹҹзҡ„й“ңдҪҚзӮ№жӣҙеҖҫеҗ‘дәҺдҝғиҝӣCOз”ҹжҲҗпјҢиҖҢдҪҚдәҺиҫ№зјҳеҢәеҹҹзҡ„й“ңдҪҚзӮ№иғҪеӨҹиҝӣдёҖжӯҘжҺЁеҠЁCO2еҗ‘з”Ізғ·пјҲCH4пјүзҡ„ж·ұеәҰиҪ¬еҢ–гҖӮеңЁеҸҜи§Ғе…үй©ұеҠЁжқЎд»¶дёӢпјҢиҜҘжқҗж–ҷиЎЁзҺ°еҮәдјҳејӮзҡ„CO2е…үеӮ¬еҢ–иҝҳеҺҹжҖ§иғҪпјҢз”Ізғ·з”ҹжҲҗж•ҲзҺҮе’ҢйҖүжӢ©жҖ§еқҮиҫҫеҲ°иҫғй«ҳж°ҙе№ігҖӮиҝӣдёҖжӯҘз ”з©¶иЎЁжҳҺпјҢжҙ»жҖ§дёӯеҝғзҡ„дҪҚзҪ®и°ғжҺ§иғҪеӨҹеҪұе“Қжқҗж–ҷеҶ…йғЁзҡ„з”өеӯҗдј йҖ’иҝҮзЁӢд»ҘеҸҠеҸҚеә”дёӯй—ҙдә§зү©зҡ„иҪ¬еҢ–иЎҢдёәпјҢд»ҺиҖҢеҶіе®ҡжңҖз»Ҳдә§зү©зұ»еһӢгҖӮиҜҘе·ҘдҪңйҰ–ж¬ЎжҸӯзӨәдәҶеӮ¬еҢ–жҙ»жҖ§дҪҚзӮ№з©әй—ҙдҪҚзҪ®еҜ№CO2иҝҳеҺҹеҸҚеә”йҖүжӢ©жҖ§зҡ„е…ій”®еҪұе“ҚпјҢдёәи®ҫи®Ўж–°еһӢй«ҳж•Ҳе…үеӮ¬еҢ–жқҗж–ҷгҖҒжҺЁеҠЁеӨӘйҳіиғҪй©ұеҠЁзҡ„з»ҝиүІеҢ–еӯҰиҪ¬еҢ–жҸҗдҫӣдәҶж–°зҡ„з ”з©¶жҖқи·ҜгҖӮ
жң¬з ”з©¶з”ұжөҷжұҹеёҲиҢғеӨ§еӯҰеҗ«ж°ҹж–°жқҗж–ҷз ”з©¶жүҖиҙІи…ҫж•ҷжҺҲеӣўйҳҹе®ҢжҲҗпјҢиҙІи…ҫж•ҷжҺҲдёәи®әж–Үзҡ„е”ҜдёҖйҖҡи®ҜдҪңиҖ…гҖӮзӣёе…із ”з©¶е·ҘдҪңеҫ—еҲ°дәҶеӣҪе®¶иҮӘз„¶з§‘еӯҰеҹәйҮ‘гҖҒжөҷжұҹзңҒиҮӘз„¶з§‘еӯҰеҹәйҮ‘зҡ„иө„еҠ©ж”ҜжҢҒгҖӮ
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